Vertical profile of tritium concentration in air during a chronic atmospheric HT release

Hiroshi Noguchi, Sumi Yokoyama

Research output: Contribution to journalArticle

Abstract

The vertical profiles of tritium gas and tritiated water concentrations in air, which would have an influence on the assessment of tritium doses as well as on the environmental monitoring of tritium, were measured in a chronic tritium gas release experiment performed in Canada in 1994. While both of the profiles were rather uniform during the day because of atmospheric mixing, large gradients of the profiles were observed at night. The gradient coefficients of the profiles were derived from the measurements. Correlations were analyzed between the gradient coefficients and meteorological conditions: solar radiation, wind speed, and turbulent diffusivity. It was found that the solar radiation was highly correlated with the gradient coefficients of tritium gas and tritiated water profiles and that the wind speed and turbulent diffusivity showed weaker correlations with those of tritiated water profiles. A one-dimensional tritium transport model was developed to analyze the vertical diffusion of tritiated water re-emitted from the ground into the atmosphere. The model consists of processes of tritium gas deposition to soil including oxidation into tritiated water, reemission of tritiated water, dilution of tritiated water in soil by rain, and vertical diffusion of tritiated water in the atmosphere. The model accurately represents the accumulation of tritiated water in soil water and the time variations and vertical profiles of tritiated water concentrations in air.

Original languageEnglish
Pages (from-to)344-353
Number of pages10
JournalHealth Physics
Volume84
Issue number3
DOIs
Publication statusPublished - 01-03-2003
Externally publishedYes

Fingerprint

Tritium
Air
Water
Gases
Soil
Atmosphere
Radiation
Rain
Environmental Monitoring
Canada

All Science Journal Classification (ASJC) codes

  • Epidemiology
  • Radiology Nuclear Medicine and imaging
  • Health, Toxicology and Mutagenesis

Cite this

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Vertical profile of tritium concentration in air during a chronic atmospheric HT release. / Noguchi, Hiroshi; Yokoyama, Sumi.

In: Health Physics, Vol. 84, No. 3, 01.03.2003, p. 344-353.

Research output: Contribution to journalArticle

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